By Ilya Prigogine, Stuart A. Rice
This sequence is dedicated to aiding the reader receive common information regarding a wide selection of issues in chemical physics, the sector of which the editors interpret very extensively. The reason is to have specialists current finished analyses of topics of curiosity and to inspire the expression of person issues of view. The editors wish that this method of the presentation of an summary of a subject matter will either stimulate new study and function a customized studying textual content for novices within the box.
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Extra resources for Advances in Chemical Physics, Vol. 77
The production of the doubly charged molecular cation by decay of the core hole is of particular interest because little is known about the properties of these ions and because the fluorescence decay DAVID M. bL 4550 4775 Figure 7. Fluoresence lines assigned to Oz2+. of the Auger final state essentially allows Auger spectroscopy to be done with the high resolution of an optical spectrometer. The first observation of dispersed luminescence following core electron excitation by monochromatic synchrotron radiation was reported for the case of oxygen (Tohji et al.
The importance of such multiple-electron excited states has been discussed for bond rupture and desorption for covalently bonded species (Ramaker 1983a, b,c; Madey et al. 1981; Jaeger et al. 1982; Treichler et al. 1985). D. Electronic localization can result from geometrical distortions or from the contraction of orbitals due to the loss of shielding by the removal of a core or valence electron. For two-hole states that result from autoionization or Auger decay of the core hole state, a more significant localization mechanism, called Coulomb localization, is present.
Nordgren, 1985, J . Chem. Phys. 83,2053. Freund, H. J. and C. M. Liegener, 1987, Chem. Phys. Lett. 134,70. , S. Svensson, H. Siegbahn, E. Basiliev, A. Faxalv, and K. Siegbahn, 1974, Chem. Phys. Lett. 28, 1. Haak, H. , G. A. Sawatzky, L. Ungier, J. K. Gimzewski, and T. D. Thomas, 1984, Rev. Sci. Instrum. 55,696. Hanson, D. , R. Stochbauer, and T. E. Madey, 1982, J. Chem. Phys. 77, 1569. Hanson, D. , S. L. Anderson, M. C. Nelson, G. P. Williams, and N. Lucas, 1985, J. Phys. Chem. 89,2235. Hayes, R.
Advances in Chemical Physics, Vol. 77 by Ilya Prigogine, Stuart A. Rice